In order for poke berries to be most useful for alternative processes, you have to get it to bind selectively to either image or non-image areas.
The experiment that left paper untouched is actually a good sign. The beautiful dyed yarn is another.
Don’t actually know how to make image or non image area attract dye though. There is oil and water in lithography, batik
/ waxed fabric and those dyed Easter eggs.
The chemists here might know what things can bind to Prussian blue, and then what things can bind to poke berry juice