Try resetting the mirror lock-up using a pointed object inserted into the reset nib on the front of the camera. Press the shutter button and wind on. MLU is part of a refined, learned technique that can be (and should be!) used in all conditions to virtually eliminate mirror/shutter whack. It's not such a good idea to use it hand-held though. Vibration from mirror and shutter travel may not be immediately visible at small sizes (or even on the lightbox), but it certainly will be visible at big enlargements of a metre or so across. Even the slightest evidence of vibration from poor technique will really, really ruin an otherwise good image.
A mirror that repeatedly jams or does not reset indicates a fault which can involve the solenoid, an archaic device that actually powers the mirror's movement (therefore when MLU is in use, get the exposure over and done with soon after activation, especially if you have a near-expired battery). Mirror return and MLU problems are common with all of the Pentax 6x7 (the earliest and oldest version dating from the 1960s) but can also effect the newer (1992->) 67 bodies. Ideally any Pentax 6x7 / 67 camera should be thoroughly tested before purchasing it. Unfortunately this just does not happen in places like eBay where just about anything goes.