I think the use of thin mica was because cellulose acetate, or nitrate film base was not invented yet, and he needed a thin transparent material so the superimposed images would register fairly well together. There have been a number of processes that create separation negatives and positives using 2 or 3 primaries to achieve a relatively complete color record. As early as the process you reference is, I am surprised he could come up with a panchromatic emulsion to shoot the negatives with.