Wiltw many thanks for your response. I can see that the 150/3.5 might not best meet my needs since at least some of the portraits will be of my young children, so the 18 x 24" FOV might be a bit large on occasion. For portraiture I agree that the 180/4 would probably be the best option. However it's a bit long for my primary landscape requirements - hence considering the 135/4 since it gives me a smaller FOV at close focus while being a focal length that I think I would use more for landscapes, but being a reasonable length for portraits (about 85mm equivalent in 135 format). I agree about the edge of frame resolution wide open, although typically this wouldn't be an issue for landscapes provided it is resolved by f/8 or so. I might be better off separating the landscape and portraiture requirement, which suggests a 135 and 180 combo, since the 150 will probably be redundant if I have both of these.
Since I currently have the 40 PE, and plan to get one of the 75s (EII or PE) next in line after the 135 or 150, this would give me a 40 / 75 / 135 / 180 set in the long term, which might be a nice combo. Thoughts?